Witnessing mass-energy equivalence with trapped atom interferometers

Jerzy Paczos1, Joshua Foo2,3,4, and Magdalena Zych1,5

1Department of Physics, Stockholm University, SE-106 91 Stockholm, Sweden
2Centre for Quantum Computation and Communication Technology, School of Mathematics and Physics, University of Queensland, St. Lucia, Queensland 4072, Australia
3Department of Physics, Stevens Institute of Technology, Castle Point Terrace, Hoboken, New Jersey 07030, USA
4Department of Physics and Astronomy, University of Waterloo, Waterloo, Ontario, Canada, N2L 3G1
5Centre for Engineered Quantum Systems, School of Mathematics and Physics, The University of Queensland, St. Lucia, Queensland, 4072, Australia

Find this paper interesting or want to discuss? Scite or leave a comment on SciRate.

Abstract

We propose an experimental setup to probe the interplay between the quantum superposition principle and gravitational time dilation arising from the mass-energy equivalence. It capitalizes on state-of-the-art atom interferometers that can keep atoms trapped in a superposition of heights in Earth's gravitational field for exceedingly long times, reaching the minute scale. Our proposal consists of adding two additional laser pulses to the existing experiments that would set up a clock trapped at a superposition of heights, reading a quantum superposition of relativistic proper times. We develop a method to include relativistic corrections to Bloch oscillations, which describe the trapped part of the interferometer. We derive the trajectories and corresponding phases acquired in each arm of the interferometer. We then show that a superposition of proper times manifests in the interference pattern in two ways: visibility modulations and a shift of the atom's resonant frequency. We argue that the latter might be observable with current technology.

State‑of‑the‑art trapped‑atom interferometers can now hold single atoms in a superposition of heights for durations comparable to a minute, while optical atomic clocks have achieved sensitivities sufficient to resolve gravitational redshifts over height differences of just a millimeter. These advances bring us closer to a regime where both quantum mechanics and general relativity are simultaneously relevant. In our proposal, we combine these capabilities by applying Ramsey interferometry to atoms trapped in a superposition of heights, effectively operating a quantum clock that experiences a superposition of proper times. When the superposed paths are recombined, this dual reading of time shows up as slow oscillations in the interference contrast and, more prominently, as a tiny shift in the clock’s resonant frequency — large enough to be within reach of today’s best atomic clocks. Experimentally demonstrating that a single atom can read out a superposition of proper times would provide direct evidence that time itself can exist in a quantum superposition. This would constitute a landmark experiment and open the door to further tests of the currently inaccessible intersection of quantum theory and relativistic gravitation.

► BibTeX data

► References

[1] A. Einstein. ``Zur elektrodynamik bewegter körper''. Annalen der physik 4 (1905).
https:/​/​doi.org/​10.1002/​andp.19053221004

[2] R. V. Pound and G. A. Rebka. ``Gravitational red-shift in nuclear resonance''. Phys. Rev. Lett. 3, 439–441 (1959).
https:/​/​doi.org/​10.1103/​PhysRevLett.3.439

[3] J. C. Hafele and R. E. Keating. ``Around-the-world atomic clocks: Predicted relativistic time gains''. Science 177, 166–168 (1972).
https:/​/​doi.org/​10.1126/​science.177.4044.166

[4] I. I. Shapiro. ``Fourth test of general relativity''. Phys. Rev. Lett. 13, 789–791 (1964).
https:/​/​doi.org/​10.1103/​PhysRevLett.13.789

[5] I. I. Shapiro, M. E. Ash, R. P. Ingalls, W. B. Smith, D. B. Campbell, R. B. Dyce, R. F. Jurgens, and G. H. Pettengill. ``Fourth test of general relativity: New radar result''. Phys. Rev. Lett. 26, 1132–1135 (1971).
https:/​/​doi.org/​10.1103/​PhysRevLett.26.1132

[6] R. Colella, A. W. Overhauser, and S. A. Werner. ``Observation of gravitationally induced quantum interference''. Phys. Rev. Lett. 34, 1472–1474 (1975).
https:/​/​doi.org/​10.1103/​PhysRevLett.34.1472

[7] M. Kasevich and S. Chu. ``Atomic interferometry using stimulated Raman transitions''. Phys. Rev. Lett. 67, 181–184 (1991).
https:/​/​doi.org/​10.1103/​PhysRevLett.67.181

[8] M. Kasevich and S. Chu. ``Measurement of the gravitational acceleration of an atom with a light-pulse atom interferometer''. Applied Physics B 54, 321–332 (1992).
https:/​/​doi.org/​10.1007/​BF00325375

[9] A. Peters, K. Y. Chung, and S. Chu. ``Measurement of gravitational acceleration by dropping atoms''. Nature 400, 849–852 (1999).
https:/​/​doi.org/​10.1038/​23655

[10] J. M. McGuirk, G. T. Foster, J. B. Fixler, M. J. Snadden, and M. A. Kasevich. ``Sensitive absolute-gravity gradiometry using atom interferometry''. Phys. Rev. A 65, 033608 (2002).
https:/​/​doi.org/​10.1103/​PhysRevA.65.033608

[11] J. B. Fixler, G. T. Foster, J. M. McGuirk, and M. A. Kasevich. ``Atom interferometer measurement of the Newtonian constant of gravity''. Science 315, 74–77 (2007).
https:/​/​doi.org/​10.1126/​science.1135459

[12] G. Lamporesi, A. Bertoldi, L. Cacciapuoti, M. Prevedelli, and G. M. Tino. ``Determination of the Newtonian gravitational constant using atom interferometry''. Phys. Rev. Lett. 100, 050801 (2008).
https:/​/​doi.org/​10.1103/​PhysRevLett.100.050801

[13] G. Rosi, F. Sorrentino, L. Cacciapuoti, M. Prevedelli, and G. M. Tino. ``Precision measurement of the Newtonian gravitational constant using cold atoms''. Nature 510, 518 (2014).
https:/​/​doi.org/​10.1038/​nature13433

[14] G. Rosi, L. Cacciapuoti, F. Sorrentino, M. Menchetti, M. Prevedelli, and G. M. Tino. ``Measurement of the gravity-field curvature by atom interferometry''. Phys. Rev. Lett. 114, 013001 (2015).
https:/​/​doi.org/​10.1103/​PhysRevLett.114.013001

[15] T. Kovachy, P. Asenbaum, C. Overstreet, C. A. Donnelly, S. M. Dickerson, A. Sugarbaker, J. M. Hogan, and M. A. Kasevich. ``Quantum superposition at the half-metre scale''. Nature 528, 530–533 (2015).
https:/​/​doi.org/​10.1038/​nature16155

[16] L. Hu, N. Poli, L. Salvi, and G. M. Tino. ``Atom interferometry with the Sr optical clock transition''. Phys. Rev. Lett. 119, 263601 (2017).
https:/​/​doi.org/​10.1103/​PhysRevLett.119.263601

[17] P. Asenbaum, C. Overstreet, M. Kim, J. Curti, and M. A. Kasevich. ``Atom-interferometric test of the equivalence principle at the ${10}^{{-}12}$ level''. Phys. Rev. Lett. 125, 191101 (2020).
https:/​/​doi.org/​10.1103/​PhysRevLett.125.191101

[18] R. Charrière, M. Cadoret, N. Zahzam, Y. Bidel, and A. Bresson. ``Local gravity measurement with the combination of atom interferometry and Bloch oscillations''. Phys. Rev. A 85, 013639 (2012).
https:/​/​doi.org/​10.1103/​PhysRevA.85.013639

[19] M. Andia, R. Jannin, F. Nez, F. Biraben, S. Guellati-Khélifa, and P. Cladé. ``Compact atomic gravimeter based on a pulsed and accelerated optical lattice''. Phys. Rev. A 88, 031605 (2013).
https:/​/​doi.org/​10.1103/​PhysRevA.88.031605

[20] X. Zhang, R. P. del Aguila, T. Mazzoni, N. Poli, and G. M. Tino. ``Trapped-atom interferometer with ultracold Sr atoms''. Phys. Rev. A 94, 043608 (2016).
https:/​/​doi.org/​10.1103/​PhysRevA.94.043608

[21] V. Xu, M. Jaffe, C. D. Panda, S. L. Kristensen, L. W. Clark, and H. Müller. ``Probing gravity by holding atoms for 20 seconds''. Science 366, 745–749 (2019).
https:/​/​doi.org/​10.1126/​science.aay6428

[22] C. D. Panda, M. Tao, J. Egelhoff, M. Ceja, V. Xu, and H. Müller. ``Coherence limits in lattice atom interferometry at the one-minute scale''. Nature Physics (2024).
https:/​/​doi.org/​10.1038/​s41567-024-02518-9

[23] S. Sinha and J. Samuel. ``Atom interferometry and the gravitational redshift''. Classical and Quantum Gravity 28, 145018 (2011).
https:/​/​doi.org/​10.1088/​0264-9381/​28/​14/​145018

[24] M. Zych, F. Costa, I. Pikovski, and Č. Brukner. ``Quantum interferometric visibility as a witness of general relativistic proper time''. Nature Communications 2 (2011).
https:/​/​doi.org/​10.1038/​ncomms1498

[25] M. Zych, F. Costa, I. Pikovski, T. C. Ralph, and Č. Brukner. ``General relativistic effects in quantum interference of photons''. Classical and Quantum Gravity 29, 224010 (2012).
https:/​/​doi.org/​10.1088/​0264-9381/​29/​22/​224010

[26] E. Castro-Ruiz, F. Giacomini, and Č. Brukner. ``Entanglement of quantum clocks through gravity''. Proceedings of the National Academy of Sciences 114, E2303–E2309 (2017).
https:/​/​doi.org/​10.1073/​pnas.1616427114

[27] S. Loriani et al. ``Interference of clocks: A quantum twin paradox''. Sci. Adv. 5, eaax8966 (2019).
https:/​/​doi.org/​10.1126/​sciadv.aax8966

[28] A. Roura. ``Gravitational redshift in quantum-clock interferometry''. Phys. Rev. X 10, 021014 (2020).
https:/​/​doi.org/​10.1103/​PhysRevX.10.021014

[29] E. Castro-Ruiz, F. Giacomini, A. Belenchia, and Č. Brukner. ``Quantum clocks and the temporal localisability of events in the presence of gravitating quantum systems''. Nat Commun 11, 2672 (2020).
https:/​/​doi.org/​10.1038/​s41467-020-16013-1

[30] A. R. H. Smith and M. Ahmadi. ``Quantum clocks observe classical and quantum time dilation''. Nat. Commun. 11, 5360 (2020).
https:/​/​doi.org/​10.1038/​s41467-020-18264-4

[31] S. Khandelwal, M. P. E. Lock, and M. P. Woods. ``Universal quantum modifications to general relativistic time dilation in delocalised clocks''. Quantum 4, 309 (2020).
https:/​/​doi.org/​10.22331/​q-2020-08-14-309

[32] P. T. Grochowski, A. R. H. Smith, A. Dragan, and K. Dębski. ``Quantum time dilation in atomic spectra''. Phys. Rev. Res. 3, 023053 (2021).
https:/​/​doi.org/​10.1103/​PhysRevResearch.3.023053

[33] J. Paczos, K. Dębski, P. T. Grochowski, A. R. H. Smith, and A Dragan. ``Quantum time dilation in a gravitational field''. Quantum 8, 1338 (2024).
https:/​/​doi.org/​10.22331/​q-2024-05-07-1338

[34] K. Dębski, P. T. Grochowski, R. Demkowicz-Dobrzański, and A. Dragan. ``Universality of quantum time dilation''. Classical and Quantum Gravity 41, 135014 (2024).
https:/​/​doi.org/​10.1088/​1361-6382/​ad4fd9

[35] P. A. Bushev, J. H. Cole, D. Sholokhov, N. Kukharchyk, and M. Zych. ``Single electron relativistic clock interferometer''. New Journal of Physics 18, 093050 (2016).
https:/​/​doi.org/​10.1088/​1367-2630/​18/​9/​093050

[36] A. Roura, C. Schubert, D. Schlippert, and E. M. Rasel. ``Measuring gravitational time dilation with delocalized quantum superpositions''. Phys. Rev. D 104, 084001 (2021).
https:/​/​doi.org/​10.1103/​PhysRevD.104.084001

[37] C. Ufrecht, F. Di Pumpo, A. Friedrich, A. Roura, C. Schubert, D. Schlippert, E. M. Rasel, W. P. Schleich, and E. Giese. ``Atom-interferometric test of the universality of gravitational redshift and free fall''. Phys. Rev. Res. 2, 043240 (2020).
https:/​/​doi.org/​10.1103/​PhysRevResearch.2.043240

[38] I. Meltzer and Y. Sagi. ``Atomic clock interferometry using optical tweezers''. Phys. Rev. A 110, 032602 (2024).
https:/​/​doi.org/​10.1103/​PhysRevA.110.032602

[39] M. Sonnleitner and S. M. Barnett. ``Mass-energy and anomalous friction in quantum optics''. Phys. Rev. A 98, 042106 (2018).
https:/​/​doi.org/​10.1103/​PhysRevA.98.042106

[40] M. Zych, Ł. Rudnicki, and I. Pikovski. ``Gravitational mass of composite systems''. Phys. Rev. D 99, 104029 (2019).
https:/​/​doi.org/​10.1103/​PhysRevD.99.104029

[41] P. K. Schwartz and D. Giulini. ``Post-Newtonian corrections to Schrödinger equations in gravitational fields''. Classical and Quantum Gravity 36, 095016 (2019).
https:/​/​doi.org/​10.1088/​1361-6382/​ab0fbd

[42] P. K. Schwartz and D. Giulini. ``Post-Newtonian Hamiltonian description of an atom in a weak gravitational field''. Phys. Rev. A 100, 052116 (2019).
https:/​/​doi.org/​10.1103/​PhysRevA.100.052116

[43] M. Zych. ``Quantum systems under gravitational time dilation''. Springer Cham. (2017).
https:/​/​doi.org/​10.1007/​978-3-319-53192-2

[44] M. Zych and Č. Brukner. ``Quantum formulation of the Einstein equivalence principle''. Nature Physics 14, 1027 (2018).
https:/​/​doi.org/​10.1038/​s41567-018-0197-6

[45] F. Di Pumpo, C. Ufrecht, A. Friedrich, E. Giese, W. P. Schleich, and W. G. Unruh. ``Gravitational redshift tests with atomic clocks and atom interferometers''. PRX Quantum 2, 040333 (2021).
https:/​/​doi.org/​10.1103/​PRXQuantum.2.040333

[46] D. E. Krause and I. Lee. ``Relativistic coupling of internal and centre of mass dynamics in classical and simple bound quantum mechanical systems''. Eur. J. Phys. 38, 045401 (2017).
https:/​/​doi.org/​10.1088/​1361-6404/​aa6903

[47] G. Tobar, S. Haine, F. Costa, and M. Zych. ``Mass-energy equivalence in gravitationally bound quantum states of the neutron''. Phys. Rev. A 106, 052801 (2022).
https:/​/​doi.org/​10.1103/​PhysRevA.106.052801

[48] V. Yudin and A. Taichenachev. ``Mass defect effects in atomic clocks''. Laser Physics Letters 15, 035703 (2018).
https:/​/​doi.org/​10.1088/​1612-202X/​aa9aa5

[49] R. Haustein, G. J. Milburn, and M. Zych. ``Mass-energy equivalence in harmonically trapped particles'' (2019). arXiv:1906.03980.
arXiv:1906.03980

[50] V. J. Martínez-Lahuerta, S. Eilers, T. E. Mehlstäubler, P. O. Schmidt, and K. Hammerer. ``Ab initio quantum theory of mass defect and time dilation in trapped-ion optical clocks''. Phys. Rev. A 106, 032803 (2022).
https:/​/​doi.org/​10.1103/​PhysRevA.106.032803

[51] A. Chu, V. J. Martínez-Lahuerta, M. Miklos, K. Kim, P. Zoller, K. Hammerer, J. Ye, and A. M. Rey. ``Exploring the dynamical interplay between mass-energy equivalence, interactions, and entanglement in an optical lattice clock''. Phys. Rev. Lett. 134, 093201 (2025).
https:/​/​doi.org/​10.1103/​PhysRevLett.134.093201

[52] T. Bothwell et al. ``Resolving the gravitational redshift across a millimetre-scale atomic sample''. Nature 602, 420–424 (2022).
https:/​/​doi.org/​10.1038/​s41586-021-04349-7

[53] X. Zheng, J. Dolde, V. Lochab, B. N. Merriman, H. Li, and S. Kolkowitz. ``Differential clock comparisons with a multiplexed optical lattice clock''. Nature 602, 425–430 (2022).
https:/​/​doi.org/​10.1038/​s41586-021-04344-y

[54] R. H. Dicke. ``The effect of collisions upon the doppler width of spectral lines''. Phys. Rev. 89, 472–473 (1953).
https:/​/​doi.org/​10.1103/​PhysRev.89.472

[55] G. Grynberg. ``Remarks on E1-E2 and E1-M1 two-photon transitions''. Journal de Physique 44, 679–682 (1983).
https:/​/​doi.org/​10.1051/​jphys:01983004406067900

[56] J. C. Bergquist, W. M. Itano, and D. J. Wineland. ``Recoilless optical absorption and doppler sidebands of a single trapped ion''. Phys. Rev. A 36, 428–430 (1987).
https:/​/​doi.org/​10.1103/​PhysRevA.36.428

[57] Tetsuya Ido and Hidetoshi Katori. ``Recoil-free spectroscopy of neutral sr atoms in the lamb-dicke regime''. Phys. Rev. Lett. 91, 053001 (2003).
https:/​/​doi.org/​10.1103/​PhysRevLett.91.053001

[58] H. Katori, M. Takamoto, V. G. Pal'chikov, and V. D. Ovsiannikov. ``Ultrastable optical clock with neutral atoms in an engineered light shift trap''. Phys. Rev. Lett. 91, 173005 (2003).
https:/​/​doi.org/​10.1103/​PhysRevLett.91.173005

[59] E. A. Alden, K. R. Moore, and A. E. Leanhardt. ``Two-photon E1-M1 optical clock''. Phys. Rev. A 90, 012523 (2014).
https:/​/​doi.org/​10.1103/​PhysRevA.90.012523

[60] G. Janson, A. Friedrich, and R. Lopp. ``Finite pulse-time effects in long-baseline quantum clock interferometry''. AVS Quantum Science 6 (2024).
https:/​/​doi.org/​10.1116/​5.0178230

[61] M. Cadoret et al. ``Atom interferometry based on light pulses: Application to the high precision measurement of the ratio h /​m and the determination of the fine structure constant''. Eur. Phys. J. Spec. Top. 172, 121 (2009).
https:/​/​doi.org/​10.1140/​epjst/​e2009-01046-2

[62] P. Storey and C. Cohen-Tannoudji. ``The Feynman path integral approach to atomic interferometry. A tutorial''. J. Phys. II France 4, 1999–2027 (1994).
https:/​/​doi.org/​10.1051/​jp2:1994103

[63] M. Werner, P. K. Schwartz, J. Kirsten-Siemß, N. Gaaloul, D. Giulini, and K. Hammerer. ``Atom interferometers in weakly curved spacetimes using Bragg diffraction and Bloch oscillations''. Phys. Rev. D 109, 022008 (2024).
https:/​/​doi.org/​10.1103/​PhysRevD.109.022008

[64] R. B. Hutson, A. Goban, G. E. Marti, L. Sonderhouse, C. Sanner, and J. Ye. ``Engineering quantum states of matter for atomic clocks in shallow optical lattices''. Phys. Rev. Lett. 123, 123401 (2019).
https:/​/​doi.org/​10.1103/​PhysRevLett.123.123401

[65] X. Zheng, J. Dolde, M. C. Cambria, H. M. Lim, and S. Kolkowitz. ``A lab-based test of the gravitational redshift with a miniature clock network''. Nat. Commun. 14, 4886 (2023).
https:/​/​doi.org/​10.1038/​s41467-023-40629-8

[66] A. Aeppli, K. Kim, W. Warfield, M. S. Safronova, and J. Ye. ``Clock with $8\times{10}^{{-}19}$ systematic uncertainty''. Phys. Rev. Lett. 133, 023401 (2024).
https:/​/​doi.org/​10.1103/​PhysRevLett.133.023401

[67] M. G. Tarallo, A. Alberti, N. Poli, M. L. Chiofalo, F.-Y. Wang, and G. M. Tino. ``Delocalization-enhanced Bloch oscillations and driven resonant tunneling in optical lattices for precision force measurements''. Phys. Rev. A 86, 033615 (2012).
https:/​/​doi.org/​10.1103/​PhysRevA.86.033615

[68] F. Bloch. ``Über die quantenmechanik der elektronen in kristallgittern''. Z. Physik 52, 555 (1929).
https:/​/​doi.org/​10.1007/​BF01339455

[69] C. Zener. ``A theory of the electrical breakdown of solid dielectrics''. Proc. R. Soc. Lond. A 145, 523 (1934).
https:/​/​doi.org/​10.1098/​rspa.1934.0116

[70] A. P. Kolchenko, S. G. Rautian, and R. I. Sokolovskii. ``Interaction of an atom with a strong electromagnetic field with the recoil effect taken into consideration''. Sov. Phys. JETP 28, 986 (1969).

[71] J. L. Hall, C. J. Bordé, and K. Uehara. ``Direct optical resolution of the recoil effect using saturated absorption spectroscopy''. Phys. Rev. Lett. 37, 1339–1342 (1976).
https:/​/​doi.org/​10.1103/​PhysRevLett.37.1339

[72] J. Ye, H. J. Kimble, and H. Katori. ``Quantum state engineering and precision metrology using state-insensitive light traps''. Science 320, 1734–1738 (2008).
https:/​/​doi.org/​10.1126/​science.1148259

[73] G. H. Wannier. ``Wave functions and effective hamiltonian for bloch electrons in an electric field''. Phys. Rev. 117, 432–439 (1960).
https:/​/​doi.org/​10.1103/​PhysRev.117.432

Cited by

[1] Abdelrahim Ruby, Wenbin Shen, Ahmed Shaker, Pengfei Zhang, Kuangchao Wu, Mostafa Ashry, and Ziyu Shen, "Next-Generation Gravitational Redshift Tests Simulated Using an Optical Link and a High-Precision Cesium Atomic Clock in Space", Universe 12 3, 82 (2026).

[2] Yiquan Yang, "Effects of gravitational time dilation on multi-photon interference", Optics Express 33 22, 46426 (2025).

[3] Gabriel Sorci, Joshua Foo, Dietrich Leibfried, Christian Sanner, and Igor Pikovski, "Quantum Signatures of Proper Time in Optical Ion Clocks", Physical Review Letters 136 16, 163602 (2026).

[4] M. F. Yassen, A.-B. A. Mohamed, A. Saad, E. K. Jaradat, and Hazrat ALi, "Gravitationally induced non-Markovianity in delocalized quantum clocks", General Relativity and Gravitation 58 3, 21 (2026).

The above citations are from Crossref's cited-by service (last updated successfully 2026-08-10 05:04:20) and SAO/NASA ADS (last updated successfully 2026-08-09 16:47:59). The list may be incomplete as not all publishers provide suitable and complete citation data.

Could not fetch ADS cited-by data during last attempt 2026-08-10 05:04:20: Cannot retrieve data from ADS due to rate limitations.